I've played all three of the games. Ar Tonelico 2 is still one of my favorite games from the PS2 era. It has one of more enjoyable and rewarding combat systems, at least for me. I actually have a review for the game up on TFF.
Anyway, the one you're talking about was a bit of a regression for me from the second. The combat was fairly enjoyable, but not as much as the last one. The main method of victory in combat is powering up your songstress and then unleashing their attack. It is generally the quickest way. But it is pretty mindless compared the second game. There is only a couple of things you have to watch out for.
The bulk of the games entertainment comes from the story and the very loosely veiled innuendos that they throw at you. Unfortunately, they sort of went a little too far on trying to provide the fan service and upping the anty that they sort of forgot the rest of what made the games so enjoyable.
Anyway, for someone that's played the last two games it is still very rewarding story wise because it is the conclusion. While you can play it independent from the others there are a lot of reference and some characters from past games that only familiar players would know. So when enjoying the story you miss out on that.
The surprising thing about the story though is that it gets pretty dark the more you play it. The girl's backgrounds and things they go through in their cosmospheres are especially dark at times. They end up going pretty edgy all things around. It was a good conclusion to the trilogy, but not the best. Two is still the best in the series.
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