I would say Mass Effect, but I believe that one is already in development, and probably being taken in the wrong direction, because female Shepherd is far more interesting than male Shepherd, but female Shepherd isn't canon, and Hollywood is sexist and hates strong female protagonists.
I could see Grand Theft Auto as a film franchise, however, if Rockstar decided to ever go in that direction, I see them writing an original story, instead of it being an adaptation of any of their games.
I think Metal Gear would make a pretty good movie. I think Uncharted would, too. And Assassin's Creed. And hell, Last Of Us was so good, they could just shoot it scene for scene, and it would be one of the best movies of all time.
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