The first time I witnessed Kefka destroying the world was pretty shocking to me. Then watching Cid die, and Celes trying to commit suicide. Then the coin toss (because I hadn't seen it earlier in the game). All of that, I saw in the same playthru, from like midnight to a bit after 2 AM, one morning way back when. I also think that 6's ending is still my favorite.
I did enjoy watching Cloud use Omnislash on Sephiroth, I must admit.
The "You're Not Alone" sequence in 9 stuck out to me, as well. As did its ending. Oh, and the Oeilvert antechamber. Holy crap.
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